Method of forming aperture plate for electron microscope

An electron microscope is described with an electron source a condenser lens having either a circular aperture for focusing a solid cone of electrons onto a specimen or an annular aperture for focusing a hollow cone of electrons onto the specimen. It also has objective lens with an annular objective aperture, for focusing electrons passing through the specimen onto an image plane. A method of making the annular objective aperture using electron imaging, electrolytic deposition and ion etching techniques is included

Structural Characterization and Gas Reactions of Small Metal Particles by High Resolution In-situ TEM and TED

A commercial electron microscope with flat-plate upper pole piece configuration of the objective lens and top entry specimen introduction was modified to obtain 5 x 10 to the minus 10th power mbar pressure at the site of the specimen while maintaining the convenience of a specimen airlock system that allows operation in the 10 to the 10th power mbar range within 15 minutes after specimen change. The specimen chamber contains three wire evaporation sources, a specimen heater, and facilities for oxygen or hydrogen plasma treatment to clean as-introduced specimens. Evacuation is achieved by dural differential pumping, with fine entrance and exit apertures for the electron beam. With the microscope operating at .000001 mbar, the first differential pumping stage features a high-speed cryopump operating in a stainless steel chamber that can be mildly baked and reaches 1 x 10 to the minus 8th power mbar. The second stage, containing the evaporation sources and a custom ionization gauge within 10 cm from the specimen, is a rigorously uncompromised all-metal uhv-system that is bakable to above 200 C throughout and is pumped with an 80-liter ion pump. Design operating pressures and image quality (resolution of metal particles smaller than 1 nm in size) was achieved

Annular objective apertures improve resolution of electron microscopes

Hollow-cone illumination techniques, using an annular objective aperture located behind back focal plane of objective lens, increase image contrast and minimize chromatic aberrations

V. The Semiclassical Foldy-Wouthuysen Transformation and the Derivation of the Bloch Equation for Spin-1/2 Polarised Beams Using Wigner Functions

A semiclassical Foldy--Wouthuysen transformation of the Dirac equation is used to obtain the radiationless Bloch equation for the polarisation density.Comment: 7 pages. No figures. Latex. Paper 5 of a set of 5. others are physics/9901038 physics/9901041 physics/9901042 physics/990104

Spin decoherence in electron storage rings --- more from a simple model

This is an addendum to the paper "Some models of spin coherence and decoherence in storage rings" by one of the authors [1] in which spin diffusion in simple electron storage rings is studied. In particular, we illustrate in a compact way, a key implication in the Epilogue of [1], namely that the exact formalism of [1] delivers a rate of depolarisation which can differ from that obtained by the conventional treatments of spin diffusion which rely on the use of the derivative $\partial \hat n/\partial\eta$ [2,3,4]. As a vehicle we consider a ring with a Siberian Snake and electron polarisation in the plane of the ring (Machine II in [1]). For this simple setup with its one-dimensional spin motion, we avoid having to deal directly with the Bloch equation [5,6] for the polarisation density. Our treatment, which is deliberately pedagogical, shows that the use of $\partial \hat n/\partial\eta$ provides a very good approximation to the rate of spin depolarisation in the model considered. But it then shows that the exact rate of depolarisation can be obtained by replacing $\partial \hat n/\partial\eta$ by another derivative as suggested in the Epilogue of [1], while giving a heuristic justification for the new derivative.Comment: 17 page

The interaction of small metal particles with refractory oxide supports

Islands and continuous layers of Pd were grown in UHV on Mo and MoO subtrates. As-deposited Pd islands and layers exhibited bulk Pd adsorption properties for CO when the Pd had been deposited at RT and at thicknesses exceeding 3 ML. However, CO adsorption was drastically reduced upon annealing. This deactivation was interpreted in terms of substrate/support interaction involving the diffusion of substrate species toward the Pd surface, using AES, TPD, and work function measurement techniques. A study of the growth and annealing behavior of Pd on Mo(110) was made for thicknesses up to 12 monolayers and substrate temperatures up to 1300K, using AES, XPS, LEED, and work function measurements. At low tempertures Pd formed a monolayer without alloying. In thick layers (12 ML) annealed about 700 K, Mo diffusion into the Pd layer and alloying were noted. Such layers remained continuous up to 1100 K. Thinner Pd layers were less stable and started coalescing upon annealing to as little as 550 K. Significant changes in Pd Auger peak shape, as well as shifts of Pd core levels, were observed during layer growth and annealing

Size and shape dependence of CO adsorption sites on sapphire supported Fe microcrystals

The surface structure and stoichiometry of alumina substrates, as well as the size, growth characteristics, and shape of Fe deposits on sapphire substrates have been investigated by low energy electron diffraction (LEED), Auger electron spectroscopy, electron energy loss spectroscopy, and X-ray photoemission spectroscopy (XPS), as well as work function measurements, in conjunction with transition electron microscopy observations. The substrates used in this work were the following: (1) new, clean Al2O3; (2) same surface amorphized by Ar ion bombardment; (3) same surface regenerated by 650 C annealing; (4) amorphous alumina films on Ta slab; and (5) polycrystal alumina films, obtained by heating amorphous films to 600 C. Substrate cleaning was found to be most effective in producing a reproducible surface upon oxygen RF plasma treatment. The Fe nucleation and growth process was found to depend strongly on the type of substrate surface and deposition conditions. Ar ion bombardment under beam flooding, and subsequent annealing at 650 C was found an effective means to restore the original Al2O3 (1102) surface for renewed Fe deposition

Direct observation of small cluster mobility and ripening

Direct evidence is reported for the simultaneous occurrence of Ostwald ripening and short-distance cluster mobility during annealing of discontinuous metal films on clean amorphous substrates. The annealing characteristics of very thin particulate deposits of silver on amorphized clean surfaces of single crystalline thin graphite substrates were studied by in-situ transmission electron microscopy (TEM) under controlled environmental conditions (residual gas pressure of 10 to the minus 9th power torr) in the temperature range from 25 to 450 C. Sputter cleaning of the substrate surface, metal deposition, and annealing were monitored by TEM observation. Pseudostereographic presentation of micrographs in different annealing stages, the observation of the annealing behavior at cast shadow edges, and measurements with an electronic image analyzing system were employed to aid the visual perception and the analysis of changes in deposit structure recorded during annealing. Slow Ostwald ripening was found to occur in the entire temperature range, but the overriding surface transport mechanism was short-distance cluster mobility

Construction of Nonlinear Symplectic Six-Dimensional Thin-Lens Maps by Exponentiation

The aim of this paper is to construct six-dimensional symplectic thin-lens transport maps for the tracking program SIXTRACK, continuing an earlier report by using another method which consistes in applying Lie series and exponentiation as described by W. Groebner and for canonical systems by A.J. Dragt. We firstly use an approximate Hamiltonian obtained by a series expansion of the square root. Furthermore, nonlinear crossing terms due to the curvature in bending magnets are neglected. An improved Hamiltonian, excluding solenoids, is introduced in Appendix A by using the unexpanded square root mentioned above, but neglecting again nonlinear crossing terms...Comment: 57 pages, late